Structural, magnetic and theoretical investigation of the magnetocaloric effect of La0.6Sr0.4MnO3/x(Sb2O3) compound

M. Nasri; J. Khelifi; J. Laifi; Fakher Hcini; Bandar Alzahrani; Mohamed Lamjed Ben Youssef Bouazizi; E. Dhahri; E. K. Hlil

doi:10.1080/01411594.2021.1927029

Structural, magnetic and theoretical investigation of the magnetocaloric effect of La_0.6Sr_0.4MnO₃/x(Sb₂O₃) compound

M. Nasri
, J. Khelifi
, J. Laifi
, Fakher Hcini
, Bandar Alzahrani
, Mohamed Lamjed Ben Youssef Bouazizi
, E. Dhahri
, E. K. Hlil

Mechanical Engineering

Research output: Contribution to journal › Article › peer-review

7 Scopus citations

Abstract

We report the structural and magnetocaloric properties of the perovskite manganite composites (La_0.6Sr_0.4MnO₃)/x(Sb₂O₃) (LSMO/Sb₂O₃) (x = 0.07 and 0.18) synthesized by the solid-state reaction method. X-ray diffraction (XRD) study was employed to confirm the formation of both the phases in composites. The results of magnetic measurements indicate that Sb₂O₃ mainly segregates at the grain boundaries of LSMO. Arrott analysis and master curve behavior reveal a second-order magnetic phase transition in the composite samples. Magnetic entropy change increases with increasing Sb₂O₃ content and a maximum of 3 J/kg. K at 2 T has been observed in the LSMO/(0.18) Sb₂O₃ sample. The enhanced ΔS_M of these composites makes them attractive for potential applications.

Original language	English
Pages (from-to)	170-182
Number of pages	13
Journal	Phase Transitions
Volume	94
Issue number	3-4
DOIs	https://doi.org/10.1080/01411594.2021.1927029
State	Published - 2021

Keywords

Composites
Hamad model
magnetic entropy change
master curve behavior

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10.1080/01411594.2021.1927029

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@article{681475a20e824bfb9df9c2631389ab45,

title = "Structural, magnetic and theoretical investigation of the magnetocaloric effect of La0.6Sr0.4MnO3/x(Sb2O3) compound",

abstract = "We report the structural and magnetocaloric properties of the perovskite manganite composites (La0.6Sr0.4MnO3)/x(Sb2O3) (LSMO/Sb2O3) (x = 0.07 and 0.18) synthesized by the solid-state reaction method. X-ray diffraction (XRD) study was employed to confirm the formation of both the phases in composites. The results of magnetic measurements indicate that Sb2O3 mainly segregates at the grain boundaries of LSMO. Arrott analysis and master curve behavior reveal a second-order magnetic phase transition in the composite samples. Magnetic entropy change increases with increasing Sb2O3 content and a maximum of 3 J/kg. K at 2 T has been observed in the LSMO/(0.18) Sb2O3 sample. The enhanced ΔSM of these composites makes them attractive for potential applications.",

keywords = "Composites, Hamad model, magnetic entropy change, master curve behavior",

author = "M. Nasri and J. Khelifi and J. Laifi and Fakher Hcini and Bandar Alzahrani and \{Ben Youssef Bouazizi\}, \{Mohamed Lamjed\} and E. Dhahri and Hlil, \{E. K.\}",

note = "Publisher Copyright: {\textcopyright} 2021 Informa UK Limited, trading as Taylor \& Francis Group.",

year = "2021",

doi = "10.1080/01411594.2021.1927029",

language = "English",

volume = "94",

pages = "170--182",

journal = "Phase Transitions",

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number = "3-4",

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TY - JOUR

T1 - Structural, magnetic and theoretical investigation of the magnetocaloric effect of La0.6Sr0.4MnO3/x(Sb2O3) compound

AU - Nasri, M.

AU - Khelifi, J.

AU - Laifi, J.

AU - Hcini, Fakher

AU - Alzahrani, Bandar

AU - Ben Youssef Bouazizi, Mohamed Lamjed

AU - Dhahri, E.

AU - Hlil, E. K.

PY - 2021

Y1 - 2021

N2 - We report the structural and magnetocaloric properties of the perovskite manganite composites (La0.6Sr0.4MnO3)/x(Sb2O3) (LSMO/Sb2O3) (x = 0.07 and 0.18) synthesized by the solid-state reaction method. X-ray diffraction (XRD) study was employed to confirm the formation of both the phases in composites. The results of magnetic measurements indicate that Sb2O3 mainly segregates at the grain boundaries of LSMO. Arrott analysis and master curve behavior reveal a second-order magnetic phase transition in the composite samples. Magnetic entropy change increases with increasing Sb2O3 content and a maximum of 3 J/kg. K at 2 T has been observed in the LSMO/(0.18) Sb2O3 sample. The enhanced ΔSM of these composites makes them attractive for potential applications.

AB - We report the structural and magnetocaloric properties of the perovskite manganite composites (La0.6Sr0.4MnO3)/x(Sb2O3) (LSMO/Sb2O3) (x = 0.07 and 0.18) synthesized by the solid-state reaction method. X-ray diffraction (XRD) study was employed to confirm the formation of both the phases in composites. The results of magnetic measurements indicate that Sb2O3 mainly segregates at the grain boundaries of LSMO. Arrott analysis and master curve behavior reveal a second-order magnetic phase transition in the composite samples. Magnetic entropy change increases with increasing Sb2O3 content and a maximum of 3 J/kg. K at 2 T has been observed in the LSMO/(0.18) Sb2O3 sample. The enhanced ΔSM of these composites makes them attractive for potential applications.

KW - Composites

KW - Hamad model

KW - magnetic entropy change

KW - master curve behavior

UR - https://www.scopus.com/pages/publications/85106208628

U2 - 10.1080/01411594.2021.1927029

DO - 10.1080/01411594.2021.1927029

M3 - Article

AN - SCOPUS:85106208628

SN - 0141-1594

VL - 94

SP - 170

EP - 182

JO - Phase Transitions

JF - Phase Transitions

IS - 3-4

ER -

Structural, magnetic and theoretical investigation of the magnetocaloric effect of La_0.6Sr_0.4MnO₃/x(Sb₂O₃) compound

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Keywords

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